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Long and Chang et al.[1] synthesized a molecular complex [MoS2]2+([(PY5Me2)MoS2]2+,PY5Me2 = 2,6-bis(1,1-bis(2-pyridyl)ethyl)pyridine)that mimics the reactive edge sites of the nanoparticulate MoS2 for the electrocatalyzed hydrogen evolution reaction(HER)at room temperature.