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The complex cation 1(Fe(bipy-NH2)3 2+),which was constructed from compound [Fe(H2Bpz2)2(bipy-NH2)] and bipy-NH2 ligands,effectively bind CO2 in-situ from a methanol-water solution,through the formation of "similar-bicarbonate" species CO2-OH-CO2 and CO2-CO2-OH.