Carbon dots, as a rising fluorescent materials have attracted continuously attention for potential applications in LED, solar cells, sensor, bioimaging and photocatalyst. However, its photo luminescent quantum yield (PL QY) is still quite low, especially emission inlong wavelength region like red light. Herein, we proposed increasing the PL QY by doped carbon dots with N or S, N. The PL QY of carbon dots dramatically rises up after doping with N. It can reach over 90%.