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Ordered mesoporous carbons without deposition of metal particles are demonstrated to be robust catalysts for direct dehydrogenation of propane without any auxiliary stream, exhibiting high activity and selectivity, as well as long catalytic stability.Their large and well-ordered porosity is advantageous for mass transport and good thermal stability, playing an important role in the catalytic performance.Our findings provide a new perspective for the application of ordered mesoporous carbon materials.