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The alignment dependence strong field ionization and dissociation builds on the alignment sensitive ionization and dissociation yields from inner and outer valence orbitals have been studied.Here, we report experiments on strong field laser interact with aligned CH3Br molecules dedicated to understood the angular dependence of ionization and dissociatior.The maximum ionization rate appears when the polarization of probe laser perpendicular to the molecular axis, but the fragment ions signal maximum when the probe laser parallel to the molecular axis.