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Two-dimensional (2D) carbon nanosheets (CNSs), which consist of few-to multi-layer of graphene sheets, have attracted great interest in many fields because of their high surface area, high height/thickness ratio, and chemical inertness.Among the various synthesis approaches for CNSs, plasma-enhanced chemical vapor deposition (PECVD) has been considered as a promising method for CNS large area production as well as low cost.