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The magnetic and dielectric properties of Sr-substituted Zn2-Y hexagonal ferrites (Ba2-xSrxZn2Fe12O22, 1.0 ≤x ≤ 1.5) are studied in this paper. Sr substitution will lead to the variation of cation occupation, which influences both the magnetic and electric properties. As Sr content x rises from 1.0 to 1.5, magnetic hysteresis loop gets wider gradually and the permeability drops rapidly due to the transformation from ferrimagnetic to antiferromagnetic phase. Moreover,permittivity rises with increasing Sr content. Under a certain exteal magnetic field, the phase transition of helical spin structure of Ba0.5Sr1.sZn2Fe12O22 at about 295 K seems to open a possibility for the room-temperature ferroelectricity induced by magnetic field. But its low resistivity prevents the observation of ferroelectric and magnetoelectric properties at room-temperature.