Graphene/SrTiO3 interface-based UV photodetectors with high responsivity

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Strontium titanate(SrTiO3),which is a crucial perovskite oxide with a direct energy band gap of 3.2 eV,holds great promise for ultraviolet(UV)photodetection.However,the response performance of the conventional SrTiO3-based pho-todetectors is limited by the large relative dielectric constant of the material,which reduces the internal electric field for electron-hole pair separation to form a current collected by electrodes.Recently,graphene/semiconductor hybrid photode-tectors by van-der-Waals heteroepitaxy method demonstrate ultrahigh sensitivity,which is benefit from the interface junc-tion architecture and then prolonged lifetime of photoexcited carriers.Here,a graphene/SrTi03 interface-based photode-tector is demonstrated with an ultrahigh responsivity of 1.2 x 106 A/W at the wavelength of 325 nm and~2.4 x 104 A/W at 261 nm.The corresponding response time is in the order of~ms.Compared with graphene/GaN interface junction-based hybrid photodetectors,~2 orders of magnitude improvement of the ultrahigh responsivity originates from a gain mechanism which correlates with the large work function difference induced long photo-carrier lifetime as well as the low background carrier density.The performance of high responsivity and fast response speed facilitates SrTiO3 material for further efforts seeking practical applications.
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