Ammonium record over the last 96 years from the Muztagata glacier in Central Asia

来源 :Chinese Science Bulletin | 被引量 : 0次 | 上传用户:gjj19901005
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As a major alkaline gas in the atmosphere, ammonia (NH3) plays an important role in atmospheric chemistry. However, there is little knowledge about NH3 variations in the Central Asia. Here we ana- lyzed the ammonium (NH+4) history recorded in an ice core from the East Pamir in Central Asia, which was drilled on the Mt. Muztagata at the elevation of 7010 m a.s.l. in 2003. The core was carefully dated and NH4+ concentration history during 1907―2002 was reconstructed. The result shows that NH4+ con- centration remained approximately constant until the 1930s after a sudden decrease at the very begin- ning of the 20th century, followed by a minimum in 1940 before increasing steadily to the peak at the end of 1990s. It is found that the annual mean NH4+ concentration was strongly associated with the Northern Hemisphere temperature, suggesting the impact of temperature on NH3 emissions in the Central Asia. Moreover, an increase of NH+4 concentration after 1940 also reflects the enhancement of NH3 emissions from anthropogenic sources such as fertilizer applications and livestock wastes in the 20th century. However, there is little knowledge about NH3 variations in the Central Asia. Here we ana- lyzed the ammonium (NH + 4) history recorded in an ice core from the East Pamir in Central Asia, which was drilled on the Mt. Muztagata at the elevation of 7010 m asl in 2003. The core was carefully dated and NH4 + concentration history was reconstructed 1907-2002. The result shows that NH4 + CONCENTRATION CONTINUED until the very end of the 1930s until the end of the 1990s. It is found that the annual average of NH4 + suggesting was impact associated with the Northern Hemisphere temperature, suggesting the impact of temperature on NH3 emissions in the Central Asia. Moreover, an increase of NH + 4 concentration after 1940 also reflects the enhancement of NH3 emissions from anthropogenic sources such as fertilizer applications and livestock wastes in the 20th century.
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