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Reaction of (MeC5H4)3Ln with HOCH2CH2NMe2 in tetrahydrofuran(THF) gives the new complexes [(MeC5H4)2Ln(μ-OCH2CH2NMe2)]2 (Ln=Sm, Y, Nd) with nitrogen functionalized μ-alkoxide ligand. The complexes were characterized by elemental analysis and IR, and [(MeC