Influence of Non-Magnetic Substitutional Atoms on Spontaneous Moment and Curie Temperature of Ce2Co1

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The structure and magnetic properties of Ce2Co17-xMx(M=Ga,Al and Si) compounds for M concentrations up to x=5 were studied by means of X-ray diffraction and magnetic measurements. The experimental results show that the Curie temperatures and Co spontaneous magnetization decrease significantly with increasing the addition of non-magnetic substitutional atoms, and that Si which has a minimum solid solubility in Ce2Co17 causes a largest reduction of Curie temperature, spontaneous magnetization and moment per Co atom compared with Ga and Al.
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