Moiré superlattice modulations in single-unit-cell FeTe films grown on NbSe2 single crystals

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Interface can be a fertile ground for exotic quantum states,including topological superconductivity,Majorana mode,fractal quantum Hall effect,unconventional superconductivity,Mott insulator,etc.Here we grow single-unit-cell (1UC)FeTe film on NbSe2 single crystal by molecular beam epitaxy (MBE) and investigate the film in-situ with a home-made cryogenic scanning tunneling microscopy (STM) and non-contact atomic force microscopy (AFM) combined system.We find different stripe-like superlattice modulations on grown FeTe film with different misorientation angles with respect to NbSe2 substrate.We show that these stripe-like superlattice modulations can be understood as moiré pattern forming between FeTe film and NbSe2 substrate.Our results indicate that the interface between FeTe and NbSe2 is atomically sharp.By STM-AFM combined measurement,we suggest that the moiré superlattice modulations have an electronic origin when the misorientation angle is relatively small (≤ 3°) and have structural relaxation when the misorientation angle is relatively large (≥ 10°).
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