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The Bose-Einstein condensation of bosonic and fermionic atoms in atomic gases was performed experimentally1-4 and predicted theoretically early5.Coupling fermionic atoms to bosonic molecules,thus this alters the quantum statistics of the atomic Fermi gas system.In the next level of matter structure,there is a neutral fermionic particle,neutron,which is similar to fermionic atoms.However,there is no object formed only with neutrons in a vast mass range of covering from a single neutron up to neutron stars on observations.Here we first show a possible way to create a new type of matter,free-neutron Bose-Einstein condensate by the ultracold free-neutron-pair Bose-Einstein condensation and then determine the neutron drip line experimentally.We found free neutrons could be cooled to ultracold neutrons with very low energy by other colder neutral atoms which are cooled by the laser.