【摘 要】
:
We find that the emission from laterally coupled quantum dots is strongly polarized along the coupled direction [110], and its polarization anisotropy can be sh
【机 构】
:
School of Physics,Northeast Normal University,130024 Changchun,China;Clarendon Laboratory,Department
论文部分内容阅读
We find that the emission from laterally coupled quantum dots is strongly polarized along the coupled direction [110], and its polarization anisotropy can be shaped by changing the orientation of the polarized excitation. When the nonresonant excitation is linearly polarized perpendicular to the coupled direction [110], excitons (X1 and X2) and local biexcitons (X1X1 and X2X2) from the two separate quantum dots (QD1 and QD2) show emission anisotropy with a small degree of polarization (10%). On the other hand, when the excitation polarization is parallel to the coupled direction [110], the polarization anisotropy of excitons, local biexcitons, and coupled biexcitons (X1X2) is enhanced with a degree of polarization of 74%. We also observed a consistent anisotropy in the time-resolved photoluminescence. The decay rate of the polarized photoluminescence intensity along the coupled direction is relatively high, but the anisotropic decay rate can be modified by changing the orientation of the polarized excitation. An energy difference is also observed between the polarized emission spectra parallel and perpendicular to the coupled direction, and it increases by up to three times by changing the excitation polarization orientation from [110] to [110]. These results suggest that the dipole–dipole interaction across the two separate quantum dots is mediated and that the anisotropic wavefunctions of the excitons and biexcitons are shaped by the excitation polarization.
其他文献
The interplay between free electrons, light, and matter offers unique prospects for space, time, and energy resolved optical material characterization, structur
Strong terahertz (THz) electric and magnetic transients open up new horizons in science and applications. We review the most promising way of achieving sub-cycl
Parallelized fluorescence imaging has been a long-standing pursuit that can address the unmet need for a comprehensive three-dimensional (3D) visualization of d
AlGaN has attracted considerable interest for ultraviolet (UV) applications. With the development of UV optoelectronic devices, abnormal carrier confinement beh
Phase and polarization singularities are important degrees of freedom for electromagnetic field manipulation. Detecting these singularities is essential for mod
Organic–inorganic halide perovskites are emerging materials for photovoltaic applications with certified power conversion efficiencies (PCEs) over 25%. Generall
The Brewster's law predicts zero reflection of p-polarization on a dielectric surface at a particular angle. However, when loss is introduced into the permittiv
Interfacial host–guest complexation offers a versatile way to functionalize nanomaterials. However, the complicated interfacial environment and trace amounts o
Limited-angle tomography of an interior volume is a challenging, highly ill-posed problem with practical implications in medical and biological imaging, manufac
Shrinking conventional optical systems to chip-scale dimensions will benefit custom applications in imaging, displaying, sensing, spectroscopy, and metrology. T