Synthesis and Crystal Structure of 2-Amino-3-cyano- 4-(3,4-dimethoxyphenyl)-4H-benzo[h]chromenes

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The title compound (C22H18N2O3) has been synthesized by the reaction of 3,4- dimethoxybenzaldehyde, malononitrile and 1-naphthol in ethanol in the presence of piperidine, and its structure was characterized by elemental analysis, IR, 1H NMR and X-ray single-crystal diffraction. The crystal belongs to monoclinic, space group C2/c with a = 24.221(6), b = 9.016(2), c = 17.003(5) ? b = 93.16(1), V = 3707(2) ?, Mr = 358.38, Z = 8, Dc = 1.284 g/cm3, m(MoKa) = 0.087 mm-1, F(000) = 1504, the final R = 0.0432 and wR = 0.1085. X-ray analysis reveals that the atoms of C(1), C(2), C(3), C(4), C(5) and O(1) form a boat-form six-membered ring in which the C(1)C(2) (1.349(3) ? is a C=C double bond. The title compound (C22H18N2O3) has been synthesized by the reaction of 3,4-dimethoxybenzaldehyde, malononitrile and 1-naphthol in ethanol in the presence of piperidine, and its structure characterized by elemental analysis, IR, 1H NMR and X-ray single The crystal belongs to monoclinic space group C2 / c with a = 24.221 (6), b = 9.016 (2), c = 17.003 (5)? ​​b = 93.16 (1), V = 3707 (2) ? = 358.38, Z = 8, Dc = 1.284 g / cm3, m (MoKa) = 0.087 mm-1, F (000) = 1504, the final R = 0.0432 and wR = 0.1085. the atoms of C (1), C (2), C (3), C (4), C (5) and O (1) form a boat-form six- membered ring in which the C 2) (1.349 (3)? Is a C = C double bond.
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