,Self-healable electroluminescent devices

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Electroluminescent (EL) devices have been extensively integrated into multi-functionalized electronic systems in the role of the vitally constituent light-emitting part.However,the lifetime and reliability of EL devices are often severely restricted by concomitant damage,especially when the strain exceeds the mechanical withstanding limit.We report a self-healable EL device by adopting a modified self-healable polyacrylic acid hydrogel as the electrode and a selfhealable polyurethane as a phosphor host to realize the first omni-layer-healable light-emitting device.The physicochemical properties of each functionalized layer can be efficiently restored after experiencing substantial catastrophic damage.As a result,the luminescent performance of the self-healable EL devices is well recovered with a high healing efficiency (83.2% for 10 healing cycles at unfixed spots,and 57.7% for 20 healing cycles at a fixed spot).In addition,inter-device healing has also been developed to realize a conceptual "LEGO"-like assembly process at the device level for light-emitting devices.The design and realization of the self-healable EL devices may revive their performance and expand their lifetime even after undergoing a deadly cut.Our self-healable EL devices may serve as model systems for electroluminescent applications of the recently developed ionically conductive healable hydrogels and dielectric polymers.
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