Hydrothermal Synthesis and X-ray Characterization of Silver(I) Complex:Diacetylthiocarbamide Silver(

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The title compound [Ag(CH3CONHC(S)NH2)2](NO3) has been prepared by hydrothermal synthesis and characterized by single-crystal X-ray diffraction. It crystallizes in mo-noclinic, space group P21/c with Mr = 406.20 (C6H12Ag N5O5S2), a = 12.0680(6), b = 6.8056(5), c = 18.0173(1) ? b = 111.383(4)u001f, V = 1377.9(2) 3, Z = 4, Dc = 1.958 g/cm3 , F(000) = 808, = 1.789 mm-1, R = 0.0361 and wR = 0.1015. Of 4185 reflections ((2)max = 55.00?, 3147 were unique (Rint = 0.0174) and 2820 with I > 2(I) were used to solve the structure. The silver(I) atom adopts V-shape geometry with the AgS bond distance of 2.4271(7) and 2.7229(9) , respectively. Seven atoms of one acetylthiocarbamide ligand are coplanar, while only four atoms of another acetylthio-carbamide ligand are fairly planar. The [Ag(CH3CONHC(S)NH2)2]+ cation and nitrate anion NO3- are connected by hydrogen bonds to form a three dimensional hydrogen bonding network.. The title compound [Ag (CH3CONHC (S) NH2) 2] (NO3) has been prepared by hydrothermal synthesis and characterized by single-crystal X- ray diffraction. It crystallizes in mo-noclinic, space group P21 / c with Mr = 406.20 (C6H12AgN5O5S2) a = 12.0680 (6) b = 6.8056 (5) c = 18.0173 (1)? B = 111.383 4 u001f V = 1377.9 2 Z = 4 Dc = 1.958 Of 4185 reflections ((2) max = 55.00 ?, 3147 were unique (Rint = 0.0174) and 2820 with I> g / cm3, F (000) = 808, = 1.789 mm-1, R = 0.0361 and wR = 0.1015. The silver (I) atom adopting V-shape geometry with the AgS bond distance of 2.4271 (7) and 2.7229 (9), respectively. Seven atoms of one acetylthiocarbamide ligand are coplanar, while The [Ag (CH3CONHC (S) NH2) 2] + cation and nitrate anion NO3- are connected by hydrogen bonds to form a three dimensional hydrogen bonding network.
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