Synthesis of a new ordered mesoporous NiMoO_4 complex oxide and its efficient catalytic performance

来源 :Journal of Energy Chemistry | 被引量 : 0次 | 上传用户:cppgreate
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Highly ordered mesoporous NiMoO4material was successfully synthesized using mesoporous silica KIT-6 as hard template via vacuum nanocasting method. The structure was characterized by means of XRD, TEM, N2adsorption-desorption, Raman and FT-IR. The mesoporous NiMoO4with the coexistence of α-NiMoO4and β-NiMoO4showed well-ordered mesoporous structure, a bimodal pore size distribution and crystalline framework. The catalytic performance of NiMoO4was investigated for oxidative dehydrogenation of propane. It is demonstrated that the mesoporous NiMoO4catalyst with more surface active oxygen species showed better catalytic performance in oxidative dehydrogenation of propane in comparison with bulk NiMoO4. Highly ordered mesoporous NiMoO4material was successfully synthesized using mesoporous silica KIT-6 as hard template via vacuum nanocasting method. The structure was characterized by means of XRD, TEM, N2adsorption-desorption, Raman and FT-IR. The mesoporous NiMoO4 with the coexistence of α- NiMoO4and β-NiMoO4showed well-ordered mesoporous structure, a bimodal pore size distribution and crystalline framework. The catalytic performance of NiMoO4was investigated for oxidative dehydrogenation of propane. It is demonstrated that the mesoporous NiMoO4catalyst with more surface active oxygen species showed better catalytic performance in oxidative dehydrogenation of propane in comparison with bulk NiMoO4.
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