【摘 要】
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Metal halide perovskites have received considerable attention in the field of electroluminescence,and the external quantum efficiency of perovskite lightemittin
【机 构】
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Institute of Luminescent Materials and Information Displays, College of Materials Science and Engine
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Metal halide perovskites have received considerable attention in the field of electroluminescence,and the external quantum efficiency of perovskite lightemitting diodes has exceeded 20%.CH3NH3PbBr3 has been intensely investigated as an emitting layer in perovskite light-emitting diodes.However,perovskite films comprising CH3NH3PbBr3 often exhibit low surface coverage and poor crystallinity,leading to high current leakage,severe nonradiative recombination,and limited device performance.Herein,we demonstrate a rationale for composition engineering to obtain high-quality perovskite films.We first reduce pinholes by adding excess CH3NH3Br to the actual CH3NH3PbBr3 films,and we then add CsBr to improve the crystalline quality and to passivate nonradiative defects.As a result,the (CH3NH3)1-xCsxPbBr3 based perovskite light-emitting diodes exhibit significantly improved external quantum and power efficiencies of 6.97% and 25.18 lm/W,respectively,representing an improvement in performance dozens of times greater than that of pristine CH3NH3PbBr3-based perovskite light-emitting diodes.Our study demonstrates that composition engineering is an effective strategy for enhancing the device performance of perovskite light-emitting diodes.
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