【摘 要】
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To reduce the greenhouse effect caused by the surgery of nitrogen-oxides concentration in the atmo-sphere and develop a future energy carrier of renewables,it is very critical to develop more efficient,controllable,and highly sensitive catalytic materials
【机 构】
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Shaanxi Key Laboratory of Optoelectronic Functional Materials and Devices,School of Materials Scienc
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To reduce the greenhouse effect caused by the surgery of nitrogen-oxides concentration in the atmo-sphere and develop a future energy carrier of renewables,it is very critical to develop more efficient,controllable,and highly sensitive catalytic materials.In our work,we proposed that nitric oxide (NO),as a supplement to N2 for the synthesis of ammonia,which is equipped with a lower barrier.And the study highlighted the potential of CeO2 (111) nanosheets with La doping and oxygen vacancy (OV) as a high-performance,controllable material for NO capture at the site of Vo site,and separation the process of hy-drogenation.We also reported that the Eads of-1.12 eV with horizontal adsorption and the Bader charge of N increasing of 0.53|e| and O increasing of 0.17|e| at the most active site of reduction-OV predicted.It is worth noting that △G of NORR (NO reduction reaction) shows good performance (thermodynam-ically spontaneous reaction) to synthesize ammonia and water at room temperature in the theoretical calculation.
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钱伟长(1912年10月9日—2010年7月30日),祖籍江苏无锡,1952年加入中国民主同盟.1955年被选聘为中国科学院学部委员(院士).1956年1月—1957年5月任中国科学院力学研究所副所长.曾任中国人民政治协商会议第六届、七届、八届、九届全国政协副主席,中国民主同盟第五届、六届、七届中央委员会副主席,第七届、八届、九届名誉主席,中国力学学会第一、二届副理事长.长期从事力学研究,在板壳问题、广义变分原理、环壳解析解和汉字宏观字型编码等方面作出突出贡献.
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