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Treatment of indolyl-3-aldimines(3-tBuN=CH)C8H5NH with AlMe3 afforded the deprotonated indolyl aluminum complex cis-[(μ-η1:η1-3-tBuN=CH)C8H5NAlMe2]2,and its crystal structure was determined by X-ray single-crystal diffraction.The crystal belongs to the or