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Chiral mesoporous inorganic materials with ordered mesostructure and single helical pore were synthesized by cooperative self-assembly of chiral templates and inorganic precursors.(i) The chiral mesoporous silica (CMS) synthesized with amino acid derived amphiphiles exhibits a novel chiral mesostructure with hexagonally ordered chiral channels twisted from the two-dimensional hexagonal p6mm.Chiroptical properties of CMS material have been achieved by dispersing achiral Ag isotropic spheric nanoparticles (AgNPs) and anisotropic nanowires (AgNWs) into CMS.