Hydrothermal Synthesis and Structure of a New Molybdenum Phosphate: (NH_3CH_2CH_2NH_3)_(2.5)[Mo_5O_

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The title compound (C5N5H41P2Mo5O30.5) was synthesized under hydrothermal condition and its crystal structure was determined by X-ray diffraction. It belongs to triclinic system, space group P , with a=9.9645(6), b=10.8666(7), c=15.814(1)? α=71.482(3), β=88.528(2), γ=78.448(2)°, V=1589.4(2)3, Dc=2.510g/cm3, Z=2,μ=2.138mm-1,λ(MoKα) = 0.71073 ? F(000)=1180. The final R and wR were 0.0396 and 0.1052 for 6626 observed reflections with I ≥2σ(I), respectively. The result of the structure analysis indicates that the [Mo5O15(PO4) (HPO4)]5- anion in the title compound consists of five edge-sharing or corner-sharing MoO6 octahedra and two corner-sharing PO4 tetrahedra. Each MoO6 octahedron adopts distorted octahedral geometry. It belongs to triclinic system, space group P, with a = 9.9645 (6), b = 10.8666 (7), and its crystal structure is determined by X-ray diffraction β = 88.528 (2), γ = 78.448 (2) °, V = 1589.4 (2) 3, Dc = 2.510 g / cm 3, Z = 2, μ = 2.138 mm-1, λ (MoKα) = 0.71073 μF (000) = 1180. The final of the structure R and wR were 0.0396 and 0.1052 for 6626 observed reflections with I ≥ 2σ (I), respectively. the [Mo5O15 (PO4) (HPO4)] 5-anion in the title compound consists of five edge-sharing or corner-sharing MoO6 octahedra and two corner-sharing PO4 tetrahedra. Each MoO6 octahedron treatments distorted octahedral geometry.
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