Effects of post-annealing on crystalline and transport properties of Bi2Te3 thin films

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A well-established method is highly desirable for growing topological insulator thin films with low carrier density on a wafer-level scale.Here,we present a simple,scalable method based on magnetron sputtering to obtain high-quality Bi2Te3 films with the cartier density down to 4.0 × 1013 cm-2.In contrast to the most-used method of high substrate temperature growth,we firstly sputtered Bi2Te3 thin films at room temperature and then applied post-annealing.It enables the growth of highly-oriented Bi2Te3 thin films with larger grain size and smoother interface.The results of electrical transport show that it has a lower carrier density as well as a larger coherent length (~ 228 nm,2 K).Our studies pave the way toward large-scale,cost-effective production of Bi2Te3 thin films to be integrated with other materials in wafer-level scale for electronic and spintronic applications.
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