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Two thiouronium iodide salts,(E)-2-methyl-1,3-diphenylisothiouronium iodide(1) and 1,3-dibenzyl-2-methylisothiouronium iodide(2),were synthesized and characterized by single-crystal X-ray diffraction,1H NMR,IR,UV-vis and luminescence spectra.Single-crysta