The Nagercoil block is the southernmost crustal segment of the Southern Granulite Terrane (SGT) in India and is mainly composed of charnockitic rocks and felsic gneisses (charnockite suite). In this study, we present petro-logic, geochemical, zircon U–Pb, REE, and Hf isotopic studies on the charnockites and leucogneiss from the Nagercoil block. Based on field investigations and petrologic studies, the charnockites can be divided into garnet-bearing and garnet-absent anhydrous granulite facies rocks with orthopyroxene. The charnockites and leucogneiss show transition from adakites to non-adakitic magmatic rocks, with enrichment in LREEs (light rare earth elements) and LILEs (large ion lithophile elements), and depletion in HREEs (heavy rare earth ele-ments) and HFSEs (high field strength elements). Some of the charnockites and the leucogneiss show typical HSA (high silica adakite) characters, (high SiO2, Al2O3, Ba–Sr, La/Yb, and Sr/Y). The HSA is considered to have formed from the interaction of slab derived melts and peridotitic mantle wedge. The high Ba–Sr features were possibly inherited from subducted oceanic crust melting under high thermal gradient during Precambrian. The magmas were underplated and subjected to fractional crystallization. Zircon grains from the charnockite and leucogneiss show zoned magmatic cores surrounded by structureless metamorphic rims. Magmatic zircon grains from the charnockites show ages ranging from 1983 ± 8.8 Ma to 2046 ± 14 Ma, and the metamorphic domains show an age range of 502 ± 14 Ma to 547 ± 8.7 Ma. Zircon from the leucogneiss yielded magmatic and metamor-phic ages of 1860 ± 20 Ma and 575.6 ± 8.8 Ma. Both charnockites and leucogneiss show two prominent age peaks at 1987 Ma and 568 Ma. The REE data of the zircon grains show LREE depletion and HREE enrichment, with the metamorphic grains showing more depletion in HREE. Zircon Hf isotopic data of the magmatic cores of zircon grains from the charnockite yieldedεHf(t) values from?1.17 to 0.46 with TDM and TDMC and age peaks at 2392 Ma and 2638 Ma, suggesting Neoarchean to Paleoproterozoic juvenile sources. We suggest that the high Ba–Sr adakitic charnockite suite from the Nagercoil block formed in a Paleoproterozoic magmatic arc setting during the assembly of the Columbia supercontinent, and underwent high-grade metamorphism associated with the amalgamation of the Gondwana supercontinent during the late Neoproterozoic–Cambrian. Our study provides new insights into the vestiges of Columbia fragments within the Gondwana assembly with two distinct cycles of crustal evolution.