Nanosized Nickel Oxides Derived from the Citrate Gel Process and Performances for Electrochemical Ca

来源 :Journal of Wuhan University of Technology(Materials Science | 被引量 : 0次 | 上传用户:cainong_111
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Nanosized nickel oxide powders were prepared by thermal decomposition of the nickel citrate gel precursors. The thermal decomposition and powder materials derived from calcination of these gel precur-sors with various ratios of citric acid (CA) to nickel at different temperatures and times were characterized by thermal analysis(TG/DTA),scanning electron microscopy (SEM),x-ray diffraction (XRD),and measurement of specifi c surface area (BET) with porosity analyses. The optimized processing conditions of calcination tempera-ture 400 ℃ for 1 hour with the CA/Ni ratio of 1.2,were determined to produce the nanosized nickel oxide pow-ders with a high specific surface area of 181 m2/g,nanometer particle sizes of 15-25 nm,micro-pore diameter distribution between 4-10 nm. The capacitance characteristics of the nanosized nickel oxide electrode in various concentrations of KOH solutions were studied by the cyclic voltammetry (CV) exhibiting both a double-layer capacitance and a faradaic pseudocapacitance. The nanosized nickel oxide electrode shows a high cyclic stabil-ity and is promising for high performance electrochemical capacitors. Nanosized nickel oxide powders were prepared by thermal decomposition of the nickel citrate gel precursors. The thermal decomposition and powder materials derived from calcination of these gel precur-sors with various ratios of citric acid (CA) to nickel at different temperatures and times were characterized by thermal analysis (TG / DTA), scanning electron microscopy (SEM), x-ray diffraction (XRD), and measurement of specifi c surface area (BET) with porosity analyzes. The optimized processing conditions of calcination tempera- ture at 400 ° C for 1 hour with the CA / Ni ratio of 1.2, were determined to produce the nanosized nickel oxide pow-ders with a high specific surface area of ​​181 m2 / g, nanometer particle sizes of 15-25 nm, micro-pore diameter distribution between 4- 10 nm. The capacitance characteristics of the nanosized nickel oxide electrode in various concentrations of KOH solutions were studied by the cyclic voltammetry (CV) exhibiting both a double-layer capacitance and a faradaic pseudoc The nanosized nickel oxide electrode shows a high cyclic stabil- ity and is promising for high performance electrochemical capacitors.
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