Methane Conversion Using Dielectric Barrier Discharge: Comparison with Thermal Process and Catalyst

来源 :Journal of Natural Gas Chemistry | 被引量 : 0次 | 上传用户:renren
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
The direct conversion of methane using a dielectric barrier discharge has been experimentally studied. Experiments with different values of flow rates and discharge voltages have been performed to investigate the effects on the conversion and reaction products both qualitatively and quantitatively. Experimental results indicate that the maximum conversion of methane has been 80% at an input flow rate of 5 ml/min and a discharge voltage of 4 kV. Experimental results also show that the optimum condition has occurred at a high discharge voltage and higher input flow rate. In terms of product distribution, a higher flow rate or shorter residence time can increase the selectivity for higher hydrocarbons. No hydrocarbon product was detected using the thermal method, except hydrogen and carbon. Increasing selectivity for ethane was found when Pt and Ru catalysts presented in the plasma reaction. Hydrogenation of acetylene in the catalyst surface could have been the reason for this phenomenon as the selectivity for acetylene in the products was decreasing. The direct conversion of methane using a dielectric barrier discharge has been experimentally studied. Experiments with different values ​​of flow rates and discharge have been conducted to investigate the effects on the conversion and reaction products both qualitatively and quantitatively. Experimental results indicate that the maximum conversion of methane has been 80% at an input flow rate of 5 ml / min and a discharge voltage of 4 kV. Experimental results also show that the optimum condition has occurred at a high discharge voltage and higher input flow rate. , a higher flow rate or shorter residence time can increase the selectivity for higher hydrocarbons. No hydrocarbon product was detected using the thermal method, except hydrogen and carbon. Increasing selectivity for ethane was found when Pt and Ru catalysts presented in the plasma reaction. Hydrogenation of acetylene in the catalyst surface could have been the reason for this phenomenon as the selectivity for acetylene in the products was decreasing.
其他文献
目的 观察额尔敦-乌日勒对动脉粥样硬化(AS)家兔血清中一氧化氮(NO)含量和抗氧化酶活性的影响.方法 采用喂饲高脂饲料构建家兔AS模型,将36只家兔完全随机分为4组,每组9只.正
随着教育体制的不断改革,在当前的初中科学教学过程中,除了加强学生基础知识教学工作之外,同时还要有效培养学生的学科素养.通过灵活多变的教学方式,有效激发学生学习兴趣,进
热喷涂专业的 ISO标准 ,将在近 2~ 3年内转化为我国标准 ,欢迎有关委员单位和行业同仁报名参与这些采标标准的制订工作。这是 CSBTS/TC5 7委员会对口国际标准化的工作范围。为
期刊
该文从挂篮荷载计算、施工流程、支座及临时固结施工、挂篮安装及试验、合拢段施工、模板制作安装、钢筋安装、混凝土的浇筑及养生、测量监控等方面人手,介绍了S226海滨大桥
期刊
目的 探讨关节镜下带线锚钉治疗胫骨髁间嵴骨折的效果. 方法 2004年1月~2005年1月,对12例胫骨髁间嵴骨折,在关节镜下进行复位带线锚钉固定,术后行积极的康复训练. 结果 手术时
该文从挂篮荷载计算、施工流程、支座及临时固结施工、挂篮安装及试验、合拢段施工、模板制作安装、钢筋安装、混凝土的浇筑及养生、测量监控等方面人手,介绍了S226海滨大桥
期刊
目的 总结高危腹主动脉瘤患者腔内修复术中及术后常见并发症及其处理措施.方法 回顾性分析安徽医科大学附属安徽省立医院2008年1月至2013年12月收治的58例高危肾下型腹主动脉
该文从挂篮荷载计算、施工流程、支座及临时固结施工、挂篮安装及试验、合拢段施工、模板制作安装、钢筋安装、混凝土的浇筑及养生、测量监控等方面人手,介绍了S226海滨大桥
数学知识是生活中不可缺少的重要组成部分,而数学知识的产生源自于人们的生活实践,是的,我们数学的教育教学,同样也离不开实际生活。我国著名的数学家华罗庚就曾经说过:“宇
期刊
在当前社会信息技术快速发展的背景下,社会各行业领域对计算机专业人才的需求不断提升,职高计算机专业作为面向社会输送计算机专职人才的重要场所,必须关注学生综合能力的培