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A novel N,N'-dibenzyl-benzimidazolium tetrachlorocuprate(Ⅱ) complex, [C21H19N2]2[CuCl4], was synthesized and its crystal structure was determined by X-ray diffraction. It crystallizes in monoclinic system, space group P2/c, a=1.203 9(2) nm, b=0.975