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Phytochemical investigation of the aerial parts of Baeckea frutescens resulted in the isolation of three new mono-or sesquiterpene-based meroterpenoids,frutescones S-U (1-3),and one pair of new (±)-5,7-dihydroxy-8-isobutyryl-6-methyldihydroflavonol (4).Their structures and absolute configurations were established by HR-ESI-MS,1D and 2D NMR,and quantum chemical ECD calculation.Compound 1 exhibited inhibitory effect on NO production in LPS-activated RAW 264.7 macrophages with an IC50 value being 0.81 μmol·L-1.