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The late Neoarchean metamorphosed volcanic rocks in the south Liaoning Terrane (SLT) of the east North China Craton (NCC) are mainly composed of amphibolites and felsic gneisses and can be chemically classified as basalt (Group#1), basaltic andesite (Group#2), dacite (Group#3) and rhyodacite (Group#4). LA-ICP-MS zircon U–Th–Pb dating reveals that they formed at ～2.53–2.51 Ga. Group#1 samples are characterized by approxi-mately flat chondrite-normalized rare earth element (REE) patts with low (La/Yb)N ratios and a narrow range of (Hf/Sm)N ratios, and their magmatic precursors were generated by partial melting of a depleted mantle wedge weakly metasomatized by subducted slab fluids. Compared to Group#1 samples, Group#2 samples display strongly fractionated REE patts with higher (La/Yb)N ratios and more scattered (Hf/Sm)N ratios, indicative of a depleted mantle wedge that had been intensely metasomatized by slab-derived melts and fluids. Group#3 samples are characterized by high MgO and transition trace element concentrations and fractionated REE patts, which resemble typical high-Si adakites, and the magmatic precursors were derived from partial melting of a subducted oceanic slab. Group#4 samples have the highest SiO2 and the lowest MgO and transition trace element contents, and were derived from partial melting of basaltic rocks at lower crust levels. Integrating these tholeiitic to calc-alkaline volcanic rocks with the mass of contemporaneous dioritic-tonalitic-trondhjemitic-granodioritic gneisses, the late Neoarchean volcanic rocks in the SLT were most likely produced in an active continental margin. Furthermore, the affinities in lithological assemblages, metamorphism and tectonic regime among SLT, east Hebei to west Liaoning Terrane (EH–WLT), north Liaoning to south Jilin Terrane (NL–SJT), Anshan-Benxi continental nucleus (ABN) and Yishui complex (YSC) collectively indicate that an integral and much larger continental block had been formed in the late Neoarchean and the craton-scale lateral accretion was a dominantly geodynamic mechanism in the east NCC.