Kondo effect of magnetic impurities on topological Sb(111)

来源 :中国化学会第29届学术年会 | 被引量 : 0次 | 上传用户:cc51wang
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
  Topological materials have regarded as a promise matter for applications in fields of spin electronic devices and quantum information processing.Since the topological states consist of antilocalized Dirac fermions where the spin and momentum are locked,to our best knowledge,it is still fully unknown how the topological states influence the quantum transports of magnetic impurities in comparison with those orthodox metallic electronic states of noble metal surfaces.Especially,one interesting question addressed is whether the conventional Kondo effect can be observed and exactly protect the TSS from magnetic scattering when magnetic adsorbates couple to the TSS.Recently,a few theoretical calculations have predicted that a Kondo effect would take place as long as the Fermi level do not locate exactly at the Dirac point,leading to spin-polarized electronic clouds that screened the magnetic moments of local impurities and thus suppressed the backscattering of the TSS.However,on relevant experiments were reported up to now.Here we attempt to investigate the adsorption behavior of CoPc molecules and Co atoms on semimetalic Sb(111)as well as the Kondo effects relating to the topological states and these magnetic impurities.Via low temperature scanning tunneling microscopy(STM),the adsorption configurations of CoPc and Co impurities are well clarified.The CoPc molecules tend to adsorb on bridge sites of the substrate and assemble into two types of well-ordered strcutures.But deposited Co atoms randomly distribute on Sb(111)and parts of them exhibiting a weak protrusion in STM images can dip into the surface layer.In scanning tunneling spectroscopy,a sharp peak near the Fermi energy is interpreted as a fingerprint of the Kondo resonance with a Kondo temperature of 205 23K.Density functional theory calculations reveal that the protruding Co atoms are responsible for the Kondo peak and those dipped Co atoms appear as nonmagnetic impurities.By identifying the quasiparticle interference wavevectors,only the scattering channels relating to backscattering confinements are observed for both surfaces with and without the Co adsorption.It suggests that the Kondo effect fully screens those protruding magnetic impurities and thereby suppresses the backscattering of the topological surface states.
其他文献
肝癌是一种原发于肝脏的恶性肿瘤。目前治疗肝癌的药物大多具有较大的毒副作用,因此,寻找敏感性高且毒副作用小的肝癌治疗药物具有重要的意义。实验室前期研究发现鳄胆汁提取物
近年来,土壤盐渍化严重地影响了作物的产量和土地的可持续利用,探讨能有效缓解土壤盐渍化给植物造成危害的方法,对提高作物产量具有重要的科学意义。本文以两个不同品种豌豆
1997年12月3日,云南丽江古城、山西平遥古城和苏州古典园林,被联合国教产文组织收入《世界文化遗产名录》,与雅典、罗马、威尼斯等世界名城一道,成为著名的世界文化遗产的一
  目前,高放废液的安全处理与处置是制约核能可持续发展的关键,溶剂萃取法是当前从高放废液中分离锕系元素和长寿命裂变产物的主流技术.如何有效地从高放废液中分离锕系和
会议
  Studies on the structure,states,and reactivity of excess electrons(EEs)in biological media are of great significance.Although there is information about EE
会议
  The 1,2,3-triazole features a physicochemical resemblance to the amide bond,due to its planarity and strong dipole moment(~5 D).In addition,the triazole uni
会议
{P4Mo6}基多金属氧酸盐(POMs)是组建超分子的理想建筑块。由于还原型MoV中心使阴离子簇具有较高的负电荷,能够诱导更多的金属单元植入晶体骨架,同时四个伸展的{PO4}片段可以
能源是人类社会生存和发展的基本条件,针对传统化石能源面临的严峻挑战,寻求新的可再生的替代能源是当今能源发展的趋势,而氢作为优良的能源载体得到了广泛的关注。产气肠杆菌(Enterobacter aerogenes)是一种极具应用前景的兼性厌氧产氢菌,它能广泛地利用各种碳源生长,产氢速率较高,具有工业应用的潜力。本研究通过敲除NADH脱氢酶亲水性亚基的基因(nuoCDE),过表达小RNA RyhB和N
摘 要:本文分析了初中英语阅读教学中阅读策略教学不充分、不恰当的现状,展示了在略读、扫读、理解逻辑关系、分析文章结构等阅读策略教学上成功的课例,旨在说明阅读策略教学的重要性以及如何更好地开展初中英语阅读策略的教学。  关键词:阅读教学;阅读策略;渗透培养  《义务教育英语课程标准(2011版)》(中华人民共和国教育部,2012)明确指出阅读教学不仅要让学生掌握语言知识,获取文章信息,领悟文章内涵,
英语语法教学是初中英语教学中的重要一环.高效的英语语法教学不仅能够帮助学生打下良好的英语基础,而且也有助于全面提高学生的英语综合能力.在当前的“互联网+”的背景下,
期刊