二氧化硅包覆NiFe_2O_4担载Preyssler杂多酸用于合成双(二氢嘧啶酮)苯和3,4-二氢嘧啶-2(1H)-酮(英文)

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A novel magnetic acidic catalyst comprising Preyssler(H14[Na P5W30O110]) heteropoly acid support‐ed on silica coated nickel ferrite nanoparticles (Ni Fe2O4@Si O2) was prepared.The catalyst was characterized by Fourier transform infrared,scanning electron microscopy,transmission electron microscopy,X‐ray diffraction,energy dispersive spectrum,VSM and particle size neasurement.Its catalytic activity was investigated for the synthesis of bis(dihydropyrimidinone)benzene and 3,4‐dihydropyrimidin‐2(1H)‐ones derivatives by the Biginelli reaction.With the catalyst,the reac‐tions occurred in less than 1 h with good to excellent yields.More importantly,the catalyst was easily separated from the reaction mixture by an external magnet and reused at least five times without degradation in the activity. A novel magnetic acidic catalyst comprising Preyssler (H14 [Na P5W30O110]) heteropoly acid support-ed on silica coated nickel ferrite nanoparticles (Ni Fe2O4 @ Si O2) was prepared. The catalyst was characterized by Fourier transform infrared, scanning electron microscopy, transmission electron microscopy, X-ray diffraction, energy dispersive spectrum, VSM and particle size neasurement. Its catalytic activity was investigated for the synthesis of bis (dihydropyrimidinone) benzene and 3,4- dihydropyrimidin-2 (1H) -ones derivatives by the Biginelli reaction. With the catalyst, the reac-tions occurred in less than 1 h with good to excellent yields.More importantly, the catalyst was easily separated from the reaction mixture by an external magnet and reused at least five times without degradation in the activity.
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