Annealing temperature dependent catalytic water oxidation activity of iron oxyhydroxide thin films

来源 :Journal of Energy Chemistry | 被引量 : 0次 | 上传用户:liuqingq
下载到本地 , 更方便阅读
声明 : 本文档内容版权归属内容提供方 , 如果您对本文有版权争议 , 可与客服联系进行内容授权或下架
论文部分内容阅读
Nanostructured iron oxyhydroxide(Fe OOH) thin films have been synthesized using an electrodeposition method on a nickel foam(NF) substrate and effect of air annealing temperature on the catalytic performance is studied. The as-deposited and annealed thin films were characterized by X-ray diffraction(XRD),X-ray photoelectron spectroscopy(XPS), field emission scanning electron microscopy(FE-SEM) and linear sweep voltammetry(LSV) to determine their structural, morphological, compositional and electrochemical properties, respectively. The as-deposited nanostructured amorphous Fe OOH thin film is converted into a polycrystalline Fe_2O_3 with hematite crystal structure at a high temperature. The Fe OOH thin film acts as an efficient electrocatalyst for the oxygen evolution reaction(OER) in an alkaline 1 M KOH electrolyte. The film annealed at 200 °C shows high catalytic activity with an onset overpotential of 240 m V with a smaller Tafel slope of 48 m V/dec. Additionally, it needs an overpotential of 290 mV to the drive the current density of 10 m A/cm~2 and shows good stability in the 1 M KOH electrolyte solution. Nanostructured iron oxyhydroxide (Fe OOH) thin films have been synthesized using an electrodeposition method on a nickel foam (NF) substrate and effect of air annealing temperature on the catalytic performance is. The as-deposited and annealed thin films were characterized by X- ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), field emission scanning electron microscopy (FE-SEM) and linear sweep voltammetry (LSV) to determine their structural, morphological, compositional and electrochemical properties, respectively. The Fe OOH thin film acts as an efficient electrocatalyst for the oxygen evolution reaction (OER) in an alkaline 1 M KOH electrolyte. The film annealed at 200 ° C shows high catalytic activity with an onset overpotential of 240 m V with a smaller Tafel slope of 48 m V / dec. Additionally, it needs an overpo tential of 290 mV to the drive the current density of 10 m A / cm ~ 2 and shows good stability in the 1 M KOH electrolyte solution.
其他文献
2014年9月29日上午,“新金朝阳杯”全国自行车、电动自行车装配技能大赛在比德文公司多功能厅隆重举行。参加本次比赛选手是由比德文一线装配工人经选拔而出。经过两个多小时
支气管哮喘的病理生理主要表现在两个方面 :平滑肌功能异常和气道炎症。这是引起哮喘症状以及疾病加重的主要原因。要在临床上有效地控制哮喘 ,治疗上必需兼顾这两方面。现有
目的:优选艾纳香中总黄酮的提取工艺。方法:采用紫外分光光度法测定总黄酮,以提取率为考察指标,用正交设计方法优选最佳提取工艺。结果:以总黄酮提取率为考察指标,其优选工艺
在本文截稿之前,2014年的春节正一步一步地向我们走来。看看窗外,忙碌了一年的人们还在为回家做着农历癸巳年最后的一次努力。或许在此时此刻,您家的团圆饭已经上桌了,看着满
请下载后查看,本文暂不支持在线获取查看简介。 Please download to view, this article does not support online access to view profile.
数字图书馆是中学教育教学的重要资源。乌鲁木齐市第六十八中学利用数字图书馆开展读书活动、指导阅读、教师备课、优化教学、开展研究性学习、进行校本培训等,做法灵活多样,
近年来,在国家农机购置补贴政策、土地流转政策等一系列利好政策的强力推动下,一大批高性能大功率拖拉机活跃在田间地头。这些大功率拖拉机在农业生产中发挥了巨大作用,对农
由中国电化学会专业委员会主办、上海电力学院承办、复旦大学协办的第十九次全国电化学大会将于2017年12月1~4日在上海市举行,本届大会主题是“电化学与可持续发展”.具体信