Natural gas releasing simulation experiments were carried out in laboratory for researching the gas storage capacity in state of high temperature and high pressure and its gas releasing potential in process of temperature decreasing and decompression. The exiting phase state was studied through measuring gas adsorption of coal and PVT phase calculating of natural gas. Gas volume, gas molecular and isotope compositions in process of temperature decreasing and decompression were measured, natural-gas yields released from the Upper Paleozoic coal strata after later Cretaceous (K3) were calculated and the formation of the reservoir was studied combining with the geological background. The results indicate that natural gas stored in coal has still bigger releasing potential after the uplift of Upper Paleozoic strata. There exists a weak gas supply-effluent equilibrium in the reservoir of Ordos Basin, which is another possible evidence that the Upper Paleozoic gas reservoir may be a deep basin gas reservoir. Natural gas releasing simulation experiments were carried out in laboratory for researching the gas storage capacity in state of high temperature and high pressure and its gas release potential in process of temperature decreasing and decompression. The exiting phase state was studied through measuring gas adsorption of coal and Gas volume, gas molecular and isotope compositions in process of temperature decreasing and decompression were measured, natural-gas yield released from the Upper Paleozoic coal strata after later Cretaceous (K3) were calculated and the formation of the reservoir was studied combining with the geological background. The results that natural coal stored in coal has still bigger releasing potential after the uplift of Upper Paleozoic strata. There exists a weak gas supply-effluent equilibrium in the reservoir of Ordos Basin, which is another possible evidence that the Upper Paleozoic gas reservoir may be a deep bas in gas reservoir.