Synthesis of bifunctional Gd_2O_3:Eu~(3+) nanocrystals and their applications in biomedical imaging

来源 :Journal of Rare Earths | 被引量 : 0次 | 上传用户:coolyl1979
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Ultrafine Gd2O3:Eu3+ nanocrystals were successfully prepared by a simple reverse microemulsion method and subsequent calcination. Their structural, optical and magnetic properties were investigated using scanning electron microscopy(SEM), transmission electron microscopy(TEM), X-ray diffraction(XRD), Fourier transform infrared(FTIR), photoluminescence(PL), and magnetic property measurement system(MPMS). The amorphous Gd2(CO3)3:Eu3+ colloidal spheres were proved as an intermediate product, and gradually transformed into crystallized Gd2O3:Eu3+ with average diameter less than 100 nm. The paramagnetic property of the synthesized Gd2O3:Eu3+ nanocrystals were confirmed with its linear hysteresis plot(M-H). And Gd2O3:Eu3+ nanocrystals showed high contrast T1-enhancing modality due to the presence of the Gd3+ ions onto the particle surface. In addition, the application of the Gd2O3:Eu3+ nanocrystals as biotag for cell labeling was reported, red fluorescence from Eu3+ ions observed by fluorescence microscopy showed that the nanocrystals could permeate the cell membrane. Cytotoxicity studies of the Gd2O3:Eu3+ nanocrystals showed no adverse effect on cell viability, evidencing their high biological compatibility. Therefore, the nanoprobe formed from Gd2O3:Eu3+ nanocrystals provided the dual modality of optical and magnetic resonance imaging. Ultrafine Gd2O3: Eu3 + nanocrystals were successfully prepared by a simple reverse microemulsion method and subsequent calcination. Their structural, optical and magnetic properties were investigated using scanning electron microscopy (SEM), transmission electron microscopy (TEM), X-ray diffraction The amorphous Gd2 (CO3) 3: Eu3 + colloidal spheres were demonstrated as an intermediate product, and successively transformed into crystallized Gd2O3: Eu3 + with an average diameter (FMS) less than 100 nm. The paramagnetic property of the synthesized Gd2O3: Eu3 + nanocrystals were confirmed with its linear hysteresis plot (MH). And Gd2O3: Eu3 + nanocrystals showed high contrast T1-enhancing modality due to the presence of the Gd3 + ions onto the particle surface . In addition, the application of the Gd2O3: Eu3 + nanocrystals as biotag for cell labeling was reported, red fluorescence from Eu3 + ions observed by fluoresc Cytotoxicity studies of the Gd2O3: Eu3 + nanocrystals showed the high modality of optical and magnetic resonance imaging.
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